Movies
* "Sweet Transvestite (from The Rocky Horror Picture Show)" as Dr. Frank-N-Furter in *The Rocky Horror Picture Show* (1975) - This is arguably his most famous villain song, and the film itself is a cult classic.
* "The Time Warp (from The Rocky Horror Picture Show)" as Dr. Frank-N-Furter in *The Rocky Horror Picture Show* (1975) - Another iconic song from the same film, showcasing Curry's energy and stage presence.
* "There's a Light (from The Rocky Horror Picture Show)" as Dr. Frank-N-Furter in *The Rocky Horror Picture Show* (1975) - This ballad highlights Curry's vocal range and the more tender side of his character.
* "The Sun Will Come Out Tomorrow (from Annie)" as Miss Hannigan in *Annie* (1982) - While Miss Hannigan is a more comedic villain, Curry brings a unique voice and performance to the role.
Other
* "The Ballad of Sweeney Todd (from Sweeney Todd: The Demon Barber of Fleet Street)" - While Curry didn't originate this song, he performed it in the Broadway adaptation of Sweeney Todd, and his version is quite memorable.
These are just a few of the villain songs Tim Curry has sung. He's also known for his voice acting in animated films and shows, often portraying villains and characters with unique vocal styles.