* Vera-Ellen as Angela
* Peter Finch as Michael
* Hermione Baddeley as Mrs. Featherstone
* George Cole as Tony
* Miles Malleson as Uncle George
* Joan Greenwood as The Lady (uncredited)
It's important to note that this film is sometimes listed as "The Angel Who Pawned Her Harp" and sometimes as "The Angel Who Pawned Her Harp (The Girl Who Bought a Harp)". This is a common issue with older films, where different versions or titles might be used.